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A notable project she starred in the period was the bilingual drama Attahasa (2013), which depicted the story of smuggler Veerappan.
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Despite the success of her first few films, success evaded the actress and she increasingly began to act in lower profile films, with a further highly-anticipated project titled Rendavathu Padam, being indefinitely delayed. The film was later shelved, with Vijayalakshmi being replaced by Deepika Padukone when the project began again as Kochadaiiyaan (2014). The film went through production delays and was briefly re-titled as Hara, while Vijayalakshmi continued to intermittently film for scenes between 20. Having signed on after Ileana D'Cruz opted out of the role, Vijayalakshmi was expected to have an animated version of her feature in the film through motion capture technology, while she would also subsequently dub for the role. In July 2008, Vijayalakshmi signed on to portray the leading female role in Soundarya Rajinikanth's directorial debut, the animation film Sultan: The Warrior, alongside Rajinikanth.
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However, her subsequent releases including Adhe Neram Adhe Idam (2009) and Kattradhu Kalavu (2010) did not perform well at the box office. Her second film, Mysskin's crime thriller Anjathe (2008) also met with a favourable reaction from critics and audiences, with a reviewer from praising her portrayal of timid girl, while noting "Vijayalakshmi is here to stay as the sweet and lovable girl next door ". Narrating the story of a local team gully cricket team, the film went on to become a surprise critical and commercial success, effectively raising the profile of the various cast and crew members associated with the project. Vijayalakshmi began her career in the entertainment industry by hosting the show "Hello Tamizha" on the STAR Vijay channel, before being approached by her childhood friend Venkat Prabhu, to feature in an acting role in his directorial debut, Chennai 600028 (2007).